First-principles density functional theory for the structural, electronic, and phonon calculations of Ca-doped bilayer graphene
Penulis/Author
Prof. Drs. Pekik Nurwantoro, M.S., Ph.D. (1); SEFTY YUNITASARI (2); Harmon Prayogi (3); Sri Hidayati (4); Prof. Sholihun, S.Si., M.Sc., Ph.D.Sc. (5)
Tanggal/Date
2025
Kata Kunci/Keyword
Abstrak/Abstract
Density functional theory is adopted for the electronic structure and phonon calculation
of Ca-doped bilayer graphene. The AA and AB stacking configurations are simulated, and
the atoms are relaxed so that the atomic forces working on them are close to zero (5.0 ×
10−3 eV/˚ A). In the final relaxation, the symmetry of C8CaC8 is D2h for AA stacking
and CS for AB stacking. The formation energy of AA stacking (1.72 eV) is much lower
than that of AB stacking (8.07 eV). According to the electronic structure calculations,
the Dirac point shifts down from the Fermi level, indicating that the Ca atom behaves
as an n-type dopant. The calculated Fermi velocities for pristine bilayer graphene are
7.69 × 105 (AA stacking) and 7.75 × 105 m/s (AB stacking). Those for Ca-doped bilayer
graphene are 7.29 × 105 (AA stacking) and 7.22 × 105 m/s (AB stacking). Phonon
calculations revealed that considering the vibrational effect, the defect concentration is
1.4 × 1016 cm−3 in the AA stacking system. Meanwhile, concentration is deficient in the
AB stacking system due to the asymmetric defect configuration.
Rumpun Ilmu
Fisika
Bahasa Asli/Original Language
English
Level
Internasional
Status
Dokumen Karya
No
Judul
Tipe Dokumen
Aksi
1
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